Capturing ultrafast synergistic spin transition in a multifunctional hybrid spin crossover system by ultrafast optical spectroscopy and electron diffraction

Jiang, Yifeng; Hayes, Stuart; Bittmann, Simon; Sarracini, Antoine; Liu, Lai Chung; Müller-Werkmeister, Henrike M.; Wentzell, Jordan S.; Takahashi, Kazuyuki; Miyawaki, Atsuhiro; Hada, Masaki; Nakano, Shinnosuke; Koshihara, Shin-ya; Ishikawa, Tadahiko; Dwayne Miller, R. J.

Jiang, Yifeng; Hayes, Stuart; Bittmann, Simon; Sarracini, Antoine; Liu, Lai Chung; Müller-Werkmeister, Henrike M.; Wentzell, Jordan S.; Takahashi, Kazuyuki; Miyawaki, Atsuhiro; Hada, Masaki; Nakano, Shinnosuke; Koshihara, Shin-ya; Ishikawa, Tadahiko; Dwayne Miller, R. J.

2022

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Abstract

Multifunctional spin crossover (SCO) complexes provide control over electronic properties of anions. Here, we study a prototypical complex to understand ultrafast reaction pathways and transitional structures and open a way for fast responsive multi-level photoswitches.

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Title Capturing ultrafast synergistic spin transition in a multifunctional hybrid spin crossover system by ultrafast optical spectroscopy and electron diffraction